Dual metal synergy promotes electrocatalytic nitrate-to-ammonia conversion in neutral electrolyte.

Dongming Wang¹, Ruikai Qi¹, Li Deng¹, Cheng Fan¹, Lin Huang¹, Zhengjie Chen², Xiaofeng Lu³

¹Alan G. MacDiarmid Institute, College of Chemistry, Jilin University, 2699 Qianjin Street, Changchun 130012, PR China.

²Faculty of Materials Science and Energy Engineering, Shenzhen University of Advanced Technology, Shenzhen, 518107, PR China. Electronic address: zj.chen2@siat.ac.cn.

³Alan G. MacDiarmid Institute, College of Chemistry, Jilin University, 2699 Qianjin Street, Changchun 130012, PR China. Electronic address: xflu@jlu.edu.cn.

PubMed DOI

Abstract

Electrocatalytic nitrate-to-ammonia reduction represents a feasible pathway for sustainable energy and environmental remediation. Despite significant advances in nitrate reduction reaction (NO3RR), achieving satisfactory ammonia yield rates and Faraday efficiency (FE) in neutral environments remains challenging. Inspired by the enzymatic processes in nature, we have designed a tandem catalyst comp…

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