Molecular Design of Thermoresponsive Cellulose: How Graft Architecture Dictates Sol-Gel Transitions.

Shenming Tao¹, Hongchen Liu², Xuejiao Lin¹, Zhipeng Sun¹, Xijun Wang¹, Haisong Qi¹

¹State Key Laboratory of Advanced Paper Making and Paper-based Materials, South China University of Technology, Guangzhou, China.

²College of Intelligent Textile and Fabric Electronics, Zhongyuan University of Technology, Zhengzhou, China.

PubMed DOI

Abstract

The development of polysaccharide-peptoid hybrids represents a promising route toward sustainable, stimuli-responsive biomaterials. However, achieving controlled synthesis and predictable thermal transitions, particularly reversible sol-gel behavior, remains challenging. Herein, we report a systematic study on the synthesis of thermoresponsive carboxymethyl cellulose (CMC) graft polymers via the U…

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